L A Masullo, F Steiner, J Zähringer, L F Lopez, J Bohlen, L Richter, F Cole, P Tinnefeld, F D Stefani Pulsed Interleaved MINFLUX Journal Article In: Nano Letters, 21 (1), pp. 840-846, 2021, ISSN: 1530-6984. Abstract | Links @article{,
title = {Pulsed Interleaved MINFLUX},
author = {L A Masullo and F Steiner and J Z\"{a}hringer and L F Lopez and J Bohlen and L Richter and F Cole and P Tinnefeld and F D Stefani},
url = {https://doi.org/10.1021/acs.nanolett.0c04600},
doi = {10.1021/acs.nanolett.0c04600},
issn = {1530-6984},
year = {2021},
date = {2021-01-13},
journal = {Nano Letters},
volume = {21},
number = {1},
pages = {840-846},
abstract = {We introduce p-MINFLUX, a new implementation of the highly photon-efficient single-molecule localization method with a simplified experimental setup and additional fluorescence lifetime information. In contrast to the original MINFLUX implementation, p-MINFLUX uses interleaved laser pulses to deliver the doughnut-shaped excitation foci at a maximum repetition rate. Using both static and dynamic DNA origami model systems, we demonstrate the performance of p-MINFLUX for single-molecule localization nanoscopy and tracking, respectively. p-MINFLUX delivers 1\textendash2 nm localization precision with 2000\textendash1000 photon counts. In addition, p-MINFLUX gives access to the fluorescence lifetime enabling multiplexing and super-resolved lifetime imaging. p-MINFLUX should help to unlock the full potential of innovative single-molecule localization schemes.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
We introduce p-MINFLUX, a new implementation of the highly photon-efficient single-molecule localization method with a simplified experimental setup and additional fluorescence lifetime information. In contrast to the original MINFLUX implementation, p-MINFLUX uses interleaved laser pulses to deliver the doughnut-shaped excitation foci at a maximum repetition rate. Using both static and dynamic DNA origami model systems, we demonstrate the performance of p-MINFLUX for single-molecule localization nanoscopy and tracking, respectively. p-MINFLUX delivers 1–2 nm localization precision with 2000–1000 photon counts. In addition, p-MINFLUX gives access to the fluorescence lifetime enabling multiplexing and super-resolved lifetime imaging. p-MINFLUX should help to unlock the full potential of innovative single-molecule localization schemes. |
L Shani, P Tinnefeld, Y Fleger, A Sharoni, B Y Shapiro, A Shaulov, O Gang, Y Yeshurun DNA origami based superconducting nanowires Journal Article In: AIP Advances, 11 (1), pp. 015130, 2021. Links @article{,
title = {DNA origami based superconducting nanowires},
author = {L Shani and P Tinnefeld and Y Fleger and A Sharoni and B Y Shapiro and A Shaulov and O Gang and Y Yeshurun},
url = {https://doi.org/10.1063/5.0029781},
doi = {10.1063/5.0029781},
year = {2021},
date = {2021-01-01},
journal = {AIP Advances},
volume = {11},
number = {1},
pages = {015130},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
|
E Cortés, L V Besteiro, A Alabastri, A Baldi, G Tagliabue, A Demetriadou, P Narang Challenges in Plasmonic Catalysis Journal Article In: ACS Nano, 14 (12), pp. 16202-16219, 2020, ISSN: 1936-0851. Abstract | Links @article{,
title = {Challenges in Plasmonic Catalysis},
author = {E Cort\'{e}s and L V Besteiro and A Alabastri and A Baldi and G Tagliabue and A Demetriadou and P Narang},
url = {https://doi.org/10.1021/acsnano.0c08773},
doi = {10.1021/acsnano.0c08773},
issn = {1936-0851},
year = {2020},
date = {2020-12-22},
journal = {ACS Nano},
volume = {14},
number = {12},
pages = {16202-16219},
abstract = {The use of nanoplasmonics to control light and heat close to the thermodynamic limit enables exciting opportunities in the field of plasmonic catalysis. The decay of plasmonic excitations creates highly nonequilibrium distributions of hot carriers that can initiate or catalyze reactions through both thermal and nonthermal pathways. In this Perspective, we present the current understanding in the field of plasmonic catalysis, capturing vibrant debates in the literature, and discuss future avenues of exploration to overcome critical bottlenecks. Our Perspective spans first-principles theory and computation of correlated and far-from-equilibrium light\textendashmatter interactions, synthesis of new nanoplasmonic hybrids, and new steady-state and ultrafast spectroscopic probes of interactions in plasmonic catalysis, recognizing the key contributions of each discipline in realizing the promise of plasmonic catalysis. We conclude with our vision for fundamental and technological advances in the field of plasmon-driven chemical reactions in the coming years.},
keywords = {},
pubstate = {published},
tppubtype = {article}
}
The use of nanoplasmonics to control light and heat close to the thermodynamic limit enables exciting opportunities in the field of plasmonic catalysis. The decay of plasmonic excitations creates highly nonequilibrium distributions of hot carriers that can initiate or catalyze reactions through both thermal and nonthermal pathways. In this Perspective, we present the current understanding in the field of plasmonic catalysis, capturing vibrant debates in the literature, and discuss future avenues of exploration to overcome critical bottlenecks. Our Perspective spans first-principles theory and computation of correlated and far-from-equilibrium light–matter interactions, synthesis of new nanoplasmonic hybrids, and new steady-state and ultrafast spectroscopic probes of interactions in plasmonic catalysis, recognizing the key contributions of each discipline in realizing the promise of plasmonic catalysis. We conclude with our vision for fundamental and technological advances in the field of plasmon-driven chemical reactions in the coming years. |